Modulation Strategies of Cu-based Electrocatalysts for Enhancing Electrocatalytic CO2 Conversion
Springer Nature
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The electrocatalytic reduction of CO₂ into high-value multi-carbon products represents a crucial pathway toward achieving carbon neutrality and sustainable chemical production. The transition from lab-scale studies to industrial-scale implementation is imperative to bridge the gap between fundamental mechanistic insights and practical applications. This book explores the mechanistic understanding and functional design of electrocatalysts for CO₂ electroreduction, focusing on bridging the gap between lab-scale research and industrial-scale implementation. It systematically investigates the role of grain boundary structures, oxidation states, and interfacial microenvironments in stabilizing Cu-based catalysts, thereby enhancing the selective production of multi-carbon products. By integrating oxidation and alloying strategies, this work introduces new approaches to modulate copper oxidation states, leading to improved catalytic performance. Advanced characterization techniques, including in situ multimodal spectroscopy, provide insights into the electrochemical stability of Cuδ⁺ species and their impact on reaction pathways. Beyond catalyst design, this book extends the discussion…
